Robust Quantum Griffiths Singularity at above 1.5 Kelvin in Nitride Thin Films

TL;DR

This study reports the observation of a robust quantum Griffiths singularity in NbN nitride thin films at temperatures above 1.5 Kelvin, demonstrating activated scaling behavior and divergence of the dynamical critical exponent.

Contribution

It provides the first experimental evidence of a stable QGS at relatively high temperatures in nitride thin films, highlighting the role of Pauli paramagnetic effects.

Findings

Quantum Griffiths singularity observed above 1.5 K in NbN films.

Divergent dynamical critical exponent near low temperatures.

Activated scaling behavior up to 4.0 K.

Abstract

Quantum Griffiths singularity (QGS), which is closely correlated with the quenched disorder, is characterized by the divergence of the dynamical critical exponent and the presence of activated scaling behavior. Typically such a quantum phenomenon is rather rare and only observed in extremely low temperatures. Here we report the experimental observation of a robust QGS in nitride thin films, NbN, which survives in a rather high temperature range. The electrical transport propertied were measured under the magnetic field up to 12 T. The field induced superconductor-metal transitions were observed with the continuously changed transition points with the decrease of temperature. The dynamical critical exponent based on the conventional power-law scaling reveals a divergent trend when approaching the the low temperature limit. Moreover, the temperature and field dependence of sheet resistance can be described by the activated scaling analysis in the temperature region up to 1.6 K $\leq T \leq$ 4.0 K. We argue that the robustness of QGS in the present system originates from the Pauli paramagnetic effect due to the strong coupling between the magnetic field and the spin degree of freedom.