One-Dimensional Spin-Polarised Surface States -- A Comparison of Bi(112) with Other Vicinal Bismuth Surfaces

TL;DR

This study investigates one-dimensional spin-polarised surface states on Bi(112) vicinal surfaces using ARPES, theoretical models, and compares them with other bismuth surfaces, highlighting their potential for spintronic applications.

Contribution

It provides the first detailed experimental and theoretical analysis of 1D spin-polarised surface states on Bi(112), demonstrating their robustness and tunability for spintronics.

Findings

Identified two 1D spin-polarised surface states on Bi(112)

States are elongated Dirac-cones with direction-dependent dispersion

Surface states' spin-polarisation can be engineered through crystal preparation

Abstract

Vicinal surfaces of bismuth are unique test-beds for investigating one-dimensional (1D) spin-polarised surface states that may one day be used in spintronic devices. In this work, two such states have been observed for the (112) surface when measured using angle-resolved photoemission spectroscopy (ARPES) and spin-resolved ARPES, and when calculated using a tight-binding (TB) model and with density functional theory (DFT). The surface states appear as elongated Dirac-cones which are 1D and almost dispersionless in the ${k}_{\text{y}}$-direction, but disperse with energy in the orthogonal ${k}_{\text{x}}$-direction to form two ``$\times$''-like features centered at the ${k}_{\text{y}}$-line through ${\Gamma}$. Unlike many materials considered for spintronic applications, their 1D nature suggests that conductivity and spin-transport properties are highly dependent on direction. The spin-polarisation of the surface states is mainly in-plane and parallel to the 1D state, but there are signs of a tilted out-of-plane spin-component for one of them. The Bi(112) surface states resemble those found for other vicinal surfaces of bismuth, strongly indicating that their existence and general properties are robust properties of vicinal surfaces of bismuth. Furthermore, differences in the details of the states, particularly related to their spin-polarisation, suggest that spin-transport properties may be engineered simply by precise cutting and polishing of the crystal.