Magnetic damping anisotropy in the two-dimensional van der Waals material Fe$_3$GeTe$_2$ from first principles

TL;DR

This study uses first-principles calculations to analyze temperature-dependent magnetic damping and anisotropy in bulk and monolayer Fe$_3$GeTe$_2$, revealing significant surface and orientation effects relevant for spintronics.

Contribution

It provides the first detailed first-principles analysis of damping anisotropy and temperature effects in Fe$_3$GeTe$_2$, highlighting the impact of surface scattering and gating.

Findings

Bulk damping increases with temperature due to resistivity.

Single-layer damping shows weak temperature dependence.

Rotational anisotropy is significant at low temperatures and can be enhanced by gating.

Abstract

Magnetization relaxation in the two-dimensional itinerant ferromagnetic van der Waals material Fe$_3$GeTe$_2$, below the Curie temperature, is fundamentally important for applications to low-dimensional spintronics devices. We use first-principles scattering theory to calculate the temperature-dependent Gilbert damping for bulk and single-layer Fe$_3$GeTe$_2$. The calculated damping frequency of bulk Fe$_3$GeTe$_2$ increases monotonically with temperature because of the dominance of resistivitylike behavior. By contrast, a very weak temperature dependence is found for the damping frequency of a single layer, which is attributed to strong surface scattering in this highly confined geometry. A systematic study of the damping anisotropy reveals that orientational anisotropy is present in both bulk and single-layer Fe3GeTe2. Rotational anisotropy is significant at low temperatures for both the bulk and a single layer and is gradually diminished by temperature-induced disorder. The rotational anisotropy can be significantly enhanced by up to 430% in gated single-layer Fe$_3$GeTe$_2$.