An efficient low-density grating setup for monochromatization of XUV ultrafast light sources

TL;DR

This paper compares two methods for harmonic selection in ultrafast XUV light sources, demonstrating that a low-density grating setup offers higher transmission with minimal temporal broadening, aiding experimental design.

Contribution

It introduces and evaluates a low-density grating approach for harmonic selection, showing its advantages over traditional mirror+filter methods in efficiency and simplicity.

Findings

Grating approach provides 3.3 to 12.9 times higher transmission.

Temporal broadening increases by only 6.8%.

Spot size increases by approximately 30%.

Abstract

Ultrafast light sources have become an indispensable tool to access and understand transient phenomenon in material science. However, a simple and easy-to-implement method for harmonic selection, with high transmission efficiency and pulse duration conservation, is still a challenge. Here we showcase and compare two approaches for selecting the desired harmonic from a high harmonic generation source while achieving the above goals. The first approach is the combination of extreme ultraviolet spherical mirrors with transmission filters and the second approach uses a normal-incidence spherical grating. Both solutions target time- and angle-resolved photoemission spectroscopy with photon energies in the 10-20 eV range but are relevant for other experimental techniques as well. The two approaches for harmonic selection are characterized in terms of focusing quality, efficiency, and temporal broadening. It is demonstrated that a focusing grating is able to provide much higher transmission as compared to the mirror+filter approach (3.3 times higher for 10.8 eV and 12.9 times higher for 18.1 eV), with only a slight temporal broadening (6.8% increase) and a somewhat larger spot size (~30% increase). Overall, our study establishes an experimental perspective on the trade-off between a single grating normal incidence monochromator design and the use of filters. As such, it provides a basis for selecting the most appropriate approach in various fields where an easy-to-implement harmonic selection from high harmonic generation is needed.