Searching for an eco-friendly gas mixture for the ALICE Resistive Plate Chambers

TL;DR

This paper explores eco-friendly gas mixtures for ALICE RPCs, focusing on replacing high-GWP gases with low-GWP alternatives like tetrafluoropropene, and reports preliminary promising results from cosmic ray tests and aging studies.

Contribution

It introduces a new research effort to replace high-GWP gases in RPCs with environmentally friendly alternatives and presents initial performance and aging study plans.

Findings

Preliminary cosmic ray tests show promising detector performance with new gas mixtures.

Aging studies are underway using irradiation facilities to assess long-term stability.

Collaboration setup at CERN enables accelerated testing of eco-friendly RPC gases.

Abstract

The ALICE RPCs are operated with a mixture of 89.7% $C_{2}H_{2}F_{4}$, 10% i-$C_{4}H_{10}$ and 0.3% $SF_{6}$. $C_{2}H_{2}F_{4}$ and $SF_{6}$ are fluorinated greenhouse gases with a high Global Warming Potential (GWP). New European Union regulations have imposed a progressive phase-down of the production and usage of F-gases, aiming to cut down their emission by two thirds in 2030 with respect to 2014. Even though research activities are excluded from these regulations, the phase-down will inevitably increase their price and CERN is also aiming to cut down on its emissions. For these reasons it is crucial to find a more eco-friendly gas mixture for RPCs by the time of the LHC long shutdown 3, foreseen in 2026. Since $C_{2}H_{2}F_{4}$ is the main contributor to the mixture GWP, an extensive R&D process has started to replace it with tetrafluoropropene ($C_{3}H_{2}F_{4}$), due to its chemical similarity with $C_{2}H_{2}F_{4}$ and its low GWP (around 7). Preliminary tests with cosmic rays have shown promising results in terms of detector performance. The next step is to study the long-term behavior of RPCs operated with these new gas mixtures (aging studies). Since this is a subject of interest for all (and not only) the LHC experiments, a collaboration, ECOgas@GIF++, was setup to carry out joint studies. Among others, a small ALICE-like RPC was installed at the Gamma Irradiation Facility at CERN, where they are exposed to a strong radiation field, coming from a 12.5 TBq $^{137}$Cs source, which allows one to simulate many years of operation in a relatively short time. The facility also provides a muon beam at specific times of the year, which can be used to study the detector performance (e.g. efficiency and cluster size) during and after irradiation.