Topological melting of the metastable skyrmion lattice in the chiral magnet Co$_9$Zn$_9$Mn$_2$

TL;DR

This study investigates how a metastable skyrmion lattice in the chiral magnet Co$_9$Zn$_9$Mn$_2$ undergoes a topological melting process under negative magnetic fields, revealing a partial topological charge inversion and transition to magnetic bubbles.

Contribution

It provides direct experimental evidence and numerical support for the topological melting process and charge inversion in metastable skyrmion lattices, a phenomenon not previously observed in this detail.

Findings

Metastable skyrmion lattice transforms into magnetic bubbles under negative fields.

Partial topological charge inversion occurs during the transition.

The process is supported by numerical calculations and relates to topological protection.

Abstract

In a $\beta$-Mn-type chiral magnet Co$_9$Zn$_9$Mn$_2$, we demonstrate that the magnetic field-driven collapse of a room temperature metastable topological skyrmion lattice passes through a regime described by a partial topological charge inversion. Using Lorentz transmission electron microscopy, the magnetization distribution was observed directly as the magnetic field was swept antiparallel to the original skyrmion core magnetization, i.e. negative magnetic fields. Due to the topological stability of skyrmions, a direct transition of the metastable skyrmion lattice to the equilibrium helical state is avoided for increasingly negative fields. Instead, the metastable skyrmion lattice gradually transforms into giant magnetic bubbles separated by $2\pi$ domain walls. Eventually these large structures give way to form a near-homogeneously magnetized medium that unexpectedly hosts a low density of isolated skyrmions with inverted core magnetization, and thus a total topological charge of reduced size and opposite sign compared with the initial state. A similar phenomenon has been observed previously in systems hosting ordered lattices of magnetic bubbles stabilized by the dipolar interaction and called "topological melting". With support from numerical calculations, we argue that the observed regime of partial topological charge inversion has its origin in the topological protection of the starting metastable skyrmion state.