Field-Induced Partial Disorder in a Shastry-Sutherland Lattice

TL;DR

This study reveals field-induced partial magnetic disorder in BaNd2ZnS5, a Shastry-Sutherland lattice, through neutron diffraction and magnetization measurements, highlighting complex magnetic phase transitions and stripe order behavior.

Contribution

It provides the first detailed neutron diffraction analysis of field-induced partial disorder in a Shastry-Sutherland lattice, identifying specific magnetic structures and transitions.

Findings

Identification of 2-Q antiferromagnetic order below 2.9 K.

Observation of a critical field Hc ~1.7 T causing partial disorder.

Construction of an H-T phase diagram showing magnetic phase transitions.

Abstract

A 2-Q antiferromagnetic order of the ferromagnetic dimers was found below TN = 2.9 K in the Shastry-Sutherland lattice BaNd2ZnS5 by single crystal neutron diffraction. The magnetic order can be understood by the orthogonal arrangement of local Ising Nd spins, identified by polarized neutrons. A field was applied along [1 -1 0] to probe the observed metamagnetic transition in the magnetization measurement. The field decouples two magnetic sublattices corresponding to the propagation vectors q1= (0.5, 0.5, 0) and q2= (-0.5, 0.5, 0), respectively. Each sublattice shows a stripe order with a Neel-type arrangement in each single layer. The stripe order with q1 remains nearly intact up to 6 T, while the other one with q2 is suppressed at a critical field Hc ~1.7 T, indicating a partial disorder. The Hc varies with temperature and is manifested in the H-T phase diagram constructed by measuring the magnetization in BaNd2ZnS5.