Light-induced dynamics of liquid-crystalline droplets on the surface of iron-doped lithium niobate crystals

TL;DR

This study explores how laser illumination influences the behavior of liquid crystalline droplets on iron-doped lithium niobate surfaces, revealing phase-dependent dynamic phenomena driven by photovoltaic fields.

Contribution

It demonstrates phase-specific liquid droplet dynamics induced by photovoltaic effects, highlighting differences between ferroelectric and standard nematic phases under laser illumination.

Findings

Droplets outside laser spot are dragged toward illuminated area.

Inside the laser spot, droplets form tendril-like structures.

Ferroelectric nematic droplets form conical spikes and branched jet streams.

Abstract

We investigated the effect of a photovoltaic field generated on the surface of iron-doped lithium niobate crystals on droplets of a ferroelectric nematic liquid crystalline and a standard nematic liquid crystalline material deposited on this surface. When such assembly is illuminated with a laser beam, a wide range of dynamic phenomena are initiated. Droplets located outside the laser spot are dragged in the direction of the illuminated area, while droplets located inside the illuminated region tend to bridge each other and rearrange into tendril-like structures. In the ferroelectric nematic phase (NF) these processes take place via the formation of conical spikes evolving into jet streams, similar to the behavior of droplets of conventional dielectric liquids exposed to overcritical electric fields. However, in contrast to conventional liquids, the jet streams of the NF phase exhibit profound branching. In the nematic phase (N) of both the ferroelectric nematic and the standard nematic material, dynamic processes occur via smooth-edged continuous features typical for conventional liquids subjected to under-critical fields. The difference in dynamic behavior is attributed to the large increase of dielectric permittivity in the ferroelectric nematic phase with respect to the dielectric permittivity of the nematic phase.