Melting of spin ice state and development of fifth order susceptibility with magnetic field in pyrochlore Tb2Sn2O7

TL;DR

This study explores the magnetic phase transitions and higher-order susceptibility in Tb2Sn2O7, revealing a new phase linked to fifth order susceptibility under high magnetic fields, advancing understanding of frustrated magnetic systems.

Contribution

It uncovers a novel magnetic phase with fifth order susceptibility in Tb2Sn2O7 induced by magnetic fields, highlighting the role of singlet-singlet states and Zeeman energy in spin ice behavior.

Findings

Identification of a new magnetic phase at high fields

Observation of fifth order susceptibility in Tb2Sn2O7

Enhanced Zeeman energy influences higher-order moments

Abstract

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic state at low temperatures. Tb2Sn2O7 has recently attracted significant attention due to its ordered spin-ice state. Additionally, in such systems, application of external magnetic field might result in exotic magnetic states. Our current investigation on Tb2Sn2O7 reveal the presence of a new phase associated with fifth order susceptibility at low temperatures and high magnetic fields. In this compound, at zero fields, for a stabilized spin-ice state, the singlet-singlet state separated by {\delta} play an imperative role. Under magnetic fields, {\delta} increases and the Zeeman energy associated with the magnetic anisotropy is believed to get enhanced; which can be the key ingredient for evolution of higher-order moments, above 10 kOe, in this compound.