Optical non-linearities and spontaneous translational symmetry breaking in driven-dissipative moir\'e exciton-polaritons

TL;DR

This paper explores how non-local dipolar interactions in driven-dissipative moiré exciton-polaritons lead to multi-stability and symmetry breaking, revealing complex nonlinear optical behaviors in these strongly interacting systems.

Contribution

It introduces a self-consistent semi-classical model to analyze the impact of long-range interactions on the steady-state properties of moiré exciton-polaritons.

Findings

Non-local interactions induce multi-stabilities with broken translational symmetry.

Long-range interactions distort multi-photon resonances.

The developed model captures the steady-state behavior of coupled exciton-photon systems.

Abstract

Moir\'e lattices formed from semiconductor bilayers host tightly localised excitons that can simultaneously couple strongly to light and possess large electric dipole moments. This facilitates the realization of new forms of polaritons that are very strongly interacting and that have been predicted to lead to strong optical nonlinearities controlled by multi-photon resonances. Here, we investigate the role of the non-local component of the exciton-exciton (dipolar) interactions on the optical response of these strongly-interacting moir\'e exciton-polaritons under conditions of strong optical driving. We find that the non-local interactions can strongly influence the steady-state properties leading to multi-stabilities with broken translational symmetry and pronounced distortions of the multi-photon resonances. We develop a self-consistent approach to describe the steady-state solution of moir\'e excitons coupled to a cavity field, treating the long-range interaction between the excitons and the photon field at the semi-classical level.