The synergy of electromagnetic effects and thermophysical properties of metals in the formation of laser induced periodic surface structures

TL;DR

This paper investigates how electromagnetic effects and thermophysical properties influence the formation of laser-induced periodic surface structures (LIPSS) on metals, emphasizing the importance of electron dynamics alongside electromagnetic interference.

Contribution

It presents a systematic model predicting LIPSS formation on metals considering electromagnetic interference and thermophysical effects, validated through simulations on gold and stainless steel.

Findings

Electromagnetic interference contributes to LIPSS formation.

Electron diffusion and electron-phonon coupling are crucial for stable structures.

Pronounced LIPSS are feasible on stainless steel but not on gold.

Abstract

Femtosecond pulsed lasers have been widely used over the past decades for precise materials structuring at the micro- and nano- scales. In order, though, to realize efficient material processing and account for the formation of laser induced periodic surfaces structures (LIPSS), it is very important to understand the fundamental laser-matter interaction processes. A significant contribution to the LIPSS profile appears to originate from the electromagnetic fingerprint of the laser source. In this work, we follow a systematic approach to predict the pulse-by-pulse formation of LIPSS on metals due to the development of a spatially periodic energy deposition that results from the interference of electromagnetic far fields on a non-flat surface profile. On the other hand, we demonstrate that the induced electromagnetic effects, alone, are not sufficient to allow the LIPSS formation, therefore, we emphasize on the crucial role of electron diffusion and electron-phonon coupling on the formation of stable periodic structures. Gold and stainless Steel are considered as two materials to test the theoretical model while simulation results appear to confirm the experimental results that, unlike gold, fabrication of pronounced LIPSS on stainless Steel is feasible.