A two-dimensional space-time terahertz memory in bulk SrTiO3

TL;DR

This paper demonstrates a novel ultrafast space-time terahertz memory in bulk SrTiO3, utilizing its surface as a sensor for sub-picosecond switching and multi-ps polar THz recording with high spatial resolution.

Contribution

It introduces a new approach to THz memory using SrTiO3's surface properties, enabling ultrafast and high-resolution space-time data storage.

Findings

Surface of SrTiO3 acts as an ultrafast sensor for THz signals.

Achieved sub-picosecond switching via the Kerr effect.

Demonstrated multi-ps polar THz recording with sub-diffraction spatial resolution.

Abstract

Ferroelectric materials offer unprecedented ultrafast responses and are of great interest for the development of new polarizable media under the influence of an electromagnetic field. Recent research efforts have demonstrated the role of optical excitation and intense terahertz (THz) pulses in inducing a polar order and revealing a hidden phase transition in SrTiO3 (STO), respectively. Here we show that the surface of STO crystals at room temperature act as ultrafast sensors that enable sub-picosecond switching through the Kerr effect and multi-ps recording of polar THz intensity with spatial resolution below the diffraction limit through dipole alignment relaxation. The contrast sensitivity and spatial resolution achieved by in the STO sensor are significantly superior to those of present-day near-field THz sensors based on the linear Pockels effect, and more importantly, its ability to remain polarized for several picoseconds opens the door to a new strategy for building an ultrafast space-time THz memory.