Viscous Fingering Instability of Complex Fluids in a Tapered Geometry

TL;DR

This paper investigates the viscous fingering instability in complex yield-stress fluids within a tapered geometry, developing a new stability criterion that accounts for complex rheology and geometry, validated by experiments.

Contribution

It introduces a novel linear stability analysis for complex fluids in tapered geometries without assuming negligible Bingham number, extending control strategies for viscous fingering.

Findings

Derived a new stability criterion incorporating rheology and geometry.

Experimental validation shows good agreement with theoretical predictions.

Extended understanding of viscous fingering in complex fluids beyond Newtonian assumptions.

Abstract

Viscous fingering (VF) is an interfacial instability that occurs in a narrow confinement or porous medium when a less-viscous fluid pushes a more viscous one, producing finger-like patterns. Controlling the VF instability is essential to enhance the efficiency of various technological applications. However, the control of VF instability has been challenging and so far focused on simple Newtonian fluids of constant viscosity. Here, we extend to complex yield-stress fluids and examine the controlling feasibility by carrying out a linear stability analysis using a radial cell with a converging gap gradient. We avoid making the major assumption of a small Bingham number, Bn << 1, i.e., a negligible ratio of the yield to shear stress, and instead provide a new stability criterion predicting apparent complex VF. This criterion depends on not only the complex fluid's rheology, interfacial tension, and contact angle to the wetting wall, but also the gap gradient, the radius, gap-thickness, and velocity at the fluid-fluid interface. Finally, we compare this theoretical criterion to our experimental data with nitrogen pushing a complex yield-stress fluid in a taper and find good agreement.