Inverse design in nuclear quantum optics: From artificial x-ray multi-level schemes to spectral observables

TL;DR

This paper introduces an inverse design methodology for tailoring x-ray cavity systems with M"ossbauer nuclei to achieve specific quantum optical functionalities, addressing the challenge of designing cavity structures from desired spectral observables.

Contribution

It develops an extit{ab initio} inverse design approach that separates scattering signatures from microscopic level schemes, enabling precise cavity design for nuclear quantum optics applications.

Findings

Scattering observables are not unique for a given cavity structure.

The extit{ab initio} approach uniquely determines the level scheme.

Inverse design successfully realizes functionalities like electromagnetically induced transparency.

Abstract

Ensembles of M\"ossbauer nuclei embedded in thin-film cavities form a promising platform for x-ray quantum optics. A key feature is that the joint nuclei-cavity system can be considered as an artificial x-ray multi-level scheme in the low-excitation regime. Using the cavity environment, the structure and parameters of such level schemes can be tailored beyond those offered by the bare nuclei. However, so far, the direct determination of a cavity structure providing a desired quantum optical functionality has remained an open challenge. Here, we address this challenge using an inverse design methodology. As a first qualitative result, we show that the established fitting approach based on scattering observables in general is not unique, since the analysis may lead to different multi-level systems for the same cavity if based on observables in different scattering channels. Motivated by this, we distinguish between scattering signatures and the microscopic level scheme as separate design objectives, with the latter being uniquely determined by an \textit{ab initio} approach. We find that both design objectives are of practical relevance and that they complement each other regarding potential applications. We demonstrate the inverse design for both objectives using example tasks, such as realising electromagnetically induced transparency. Our results pave the way for new applications in nuclear quantum optics involving more complex x-ray cavity designs.