Hidden interplay of current-induced spin and orbital torques in bulk Fe$_3$GeTe$_2$

TL;DR

This study reveals how the interplay of spin and orbital effects in bulk Fe3GeTe2 influences spin-orbit torques, showing layer-dependent origins and implications for material design.

Contribution

It demonstrates the complex interplay of spin and orbital torques in Fe3GeTe2 and highlights the role of orbital effects in spin-orbit torque behavior.

Findings

Layer-specific hidden current-induced torques

Alternation between spin flux and orbital torques with magnetization direction

Doping-dependent evolution of switching properties

Abstract

Low crystal symmetry of magnetic van der Waals materials naturally promotes spin-orbital complexity unachievable in common magnetic materials used for spin-orbit torque switching. Here, using first-principles methods, we demonstrate that an interplay of spin and orbital degrees of freedom has a profound impact on spin-orbit torques in a prototype van der Waals ferromagnet: Fe$_3$GeTe$_2$ (FGT). While we show that bulk FGT hosts strong "hidden" current-induced torques harvested by each of its layers, we uncover that their origin alternates between the conventional spin flux torque and the so-called orbital torque as the magnetization direction is varied. A drastic difference in the behavior of the two types of torques results in a non-trivial evolution of switching properties with doping. Our findings promote the design of non-equilibrium orbital properties as the guiding mechanism for crafting the properties of spin-orbit torques in layered van der Waals materials.