Enhanced high-order harmonics through periodicity breaks: from backscattering to impurity states

TL;DR

This paper investigates how breaking periodicity in atomic chains, through impurities or vacancies, enhances high-order harmonic generation by mechanisms like backscattering and impurity-state tunneling.

Contribution

It provides a detailed numerical study of HHG enhancement mechanisms in gapped atomic chains with variable gaps, unifying impurity and vacancy effects.

Findings

Enhanced HHG observed due to backscattering and impurity-state tunneling.

Different mechanisms dominate depending on the size of the spatial gap.

The study offers insights into how periodicity breaks influence HHG in complex systems.

Abstract

Backscattering of delocalized electrons has been recently established [Phys. Rev. A 105, L041101 (2022)] as a mechanism to enhance high-order harmonic generation (HHG) in periodic systems with broken translational symmetry. Here we study this effect for a variable spatial gap in an atomic chain. Propagating the many-electron dynamics numerically, we find enhanced HHG and identify its origin in two mechanisms, depending on the gap size, either backscattering or enhanced tunneling from an impurity state. Since the gapped atomic chain exhibits both impurities and vacancies in a unified setting, it provides insight how periodicity breaks influence HHG in different scenarios.