Revealing the topological phase diagram of ZrTe$_5$ using the complex strain fields of microbubbles

TL;DR

This study combines theoretical calculations and experimental measurements to map the topological phase diagram of ZrTe$_5$, demonstrating strain-induced topological phase transitions and enabling potential device applications.

Contribution

It provides a comprehensive analysis of how complex strain fields in ZrTe$_5$ influence its topological phases, with a validated model that predicts phase transitions without fitting parameters.

Findings

Identified a strain-induced topological insulator-metal transition in ZrTe$_5$

Mapped the topological phase diagram of ZrTe$_5$ under complex strain patterns

Demonstrated the ability to control topological phases via mechanical deformation

Abstract

Topological materials host robust properties, unaffected by microscopic perturbations, owing to the global topological properties of the bulk electron system. Materials in which the topological invariant can be changed by easily tuning external parameters are especially sought after. Zirconium pentatelluride (ZrTe$_5$) is one of a few experimentally available materials that reside close to the boundary of a topological phase transition, allowing the switching of its invariant by mechanical strain. Here, we unambiguously identify a topological insulator - metal transition as a function of strain, by a combination of ab initio calculations and direct measurements of the local charge density. Our model quantitatively describes the response to complex strain patterns found in bubbles of few layer ZrTe$_5$ without fitting parameters, reproducing the mechanical deformation dependent closing of the band gap observed using scanning tunneling microscopy. We calculate the topological phase diagram of ZrTe$_5$ and identify the phase at equilibrium, enabling the design of device architectures which exploit the unique topological switching characteristics of the system.