Study of visible-light emission in pure and methane-doped liquid argon

TL;DR

This study investigates the properties and photon yields of visible-light emission in pure and methane-doped liquid argon, revealing significant differences in emission intensity and effects of methane doping relevant for particle detection applications.

Contribution

It provides detailed measurements of visible-light emission yields in pure and methane-doped liquid argon, clarifying the impact of methane doping on light emission.

Findings

Photon yield in pure liquid argon is about 200 photons/MeV for X-rays.

Photon yield drops by about an order of magnitude with 0.01-1% methane doping.

Further methane doping up to 10% does not significantly change the photon yield.

Abstract

In liquid argon TPCs for dark matter search and neutrino detection experiments, primary scintillation light is used as a prompt signal of particle scattering, being intensively produced in the vacuum ultraviolet (VUV) due to excimer emission mechanism. On the other hand, there were indications on the production of visible-light emission in liquid argon, albeit at a much lower intensity, the origin of which is still not clear. The closely related issue is visible-light emission in liquid argon doped with methane, the interest in which is due to the possible use in neutron veto detectors for those experiments. In this work we study in detail the properties of such light emission in pure liquid argon and its mixtures with methane. In particular, the absolute photon yield of visible-light emission in pure liquid argon was measured to be about 200 and 90 photon/MeV for X-rays and alpha particles respectively. In liquid argon doped with methane the photon yield dropped down significantly, by about an order of magnitude at a methane molar content varying from 0.01 to 1%, and then almost did not change when further increasing the methane content up to 10%.