Continuous variable quantum state tomography of photoelectrons
Hugo Laurell, Daniel Finkelstein-Shapiro, Christoph Dittel, Chen Guo,, Ron Demjaha, Mattias Ammitzb\"oll, Robin Weissenbilder, Lana Neori\v{c}i\'c,, Sizuo Luo, Mathieu Gisselbrecht, Cord Arnold, Andreas Buchleitner, T\"onu, Pullerits, Anne L'Huillier, David Busto

TL;DR
This paper introduces a continuous variable quantum state tomography method for photoelectrons, enabling detailed analysis of quantum coherence and entanglement in ultrafast photoionization processes.
Contribution
It presents a novel tomography protocol for electrons from atom or molecule ionization, validated against calculations and capable of revealing quantum entanglement and coherence.
Findings
Successfully benchmarks the tomography protocol against theoretical calculations.
Distills ion-photoelectron entanglement due to spin-orbit splitting.
Enables investigation of quantum properties on ultrafast timescales.
Abstract
We propose a continuous variable quantum state tomography protocol of electrons which result from the ionization of atoms or molecules by the absorption of extreme ultraviolet light pulses. Our protocol is benchmarked against a direct calculation of the quantum state of photoelectrons ejected from helium and argon in the vicinity of a Fano resonance. In the latter case, we furthermore distill ion-photoelectron entanglement due to spin-orbit splitting. This opens new routes towards the investigation of quantum coherence and entanglement properties on the ultrafast timescale.
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Taxonomy
TopicsLaser-Matter Interactions and Applications · Advanced Electron Microscopy Techniques and Applications · Spectroscopy and Quantum Chemical Studies
