Quantitative near-field characterization of surface plasmon polaritons on monocrystalline gold platelets

TL;DR

This study provides a comprehensive quantitative analysis of surface plasmon polaritons on monocrystalline gold platelets using near-field microscopy, revealing how incident angle influences SPP signals and introducing a model to extract key plasmon parameters.

Contribution

It introduces a method for fully characterizing SPPs in reflection configuration, including amplitude, phase, wavelength, and propagation length, with experimental validation and theoretical agreement.

Findings

Optimal SPP signal disentanglement at grazing incident angles

Phase shift explained by a simple model

Accurate retrieval of SPP wavelength and propagation length

Abstract

The subwavelength confinement of surface plasmon polaritons (SPPs) makes them attractive for various applications such as sensing, light generation and solar energy conversion. Near-field microscopy associated with interferometric detection allows to visualize both the amplitude and phase of SPPs. However, their full quantitative characterization in a reflection configuration is challenging due to complex wave patterns arising from the interference between several excitation channels. Here, we present near-field measurements of SPPs on large monocrystalline gold platelets in the visible spectral range. We study systematically the influence of the incident angle of the exciting light on the SPPs launched by an atomic force microscope tip. We find that the amplitude and phase signals of these SPPs are best disentangled from other signals at grazing incident angle relative to the edge of the gold platelet. Furthermore, we introduce a simple model to explain the phase shift observed between the SPP amplitude and phase profiles. Using this model, the wavelength and propagation length of the tip-launched plasmons are retrieved by isolating and fitting their signals far from the platelets edges. Our experimental results are in excellent agreement with theoretical models using gold refractive index values. The presented method to fully characterize the SPP complex wavevector could enable the quantitative analysis of polaritons occurring in different materials at visible wavelengths.