Multiphoton absorption and Rabi oscillations in armchair graphene nanoribbons

TL;DR

This paper provides an analytical framework for understanding multiphoton absorption and Rabi oscillations in armchair graphene nanoribbons under strong electric fields, revealing dependencies on ribbon width and field strength.

Contribution

It introduces explicit analytical formulas for electron-hole pair production, multiphoton absorption, and Rabi oscillation frequencies in AGNRs, highlighting the impact of electric field oscillations.

Findings

Enhanced intersubband transitions due to oscillating electric fields

Analytical results align qualitatively with numerical methods

Experimental feasibility of observing Rabi oscillations and multiphoton absorption in AGNRs

Abstract

We present an analytical approach to the problem of the multiphoton absorption and Rabi oscillations in an armchair graphene nanoribbon (AGNR) in the presence of a time-oscillating strong electric field induced by a light wave directed parallel to the ribbon axis. The two-dimensional Dirac equation for the massless electron subject to the ribbon confinement is employed. In the resonant approximation the electron-hole pair production rate, associated with the electron transitions between the valence and conduction size-quantized subbands, the corresponding multiphoton absorption coefficient and the frequency of the Rabi oscillations are obtained in an explicit form. We trace the dependencies of the above quantities on the ribbon width and electric field strength for both the multiphoton assisted and tunneling regimes relevant to the time-oscillating and practically constant electric field, respectively. A significant enhancement effect of the oscillating character of the electric field on the intersubband transitions is encountered. Our analytical results are in qualitative agreement with those obtained for the graphene layer by numerical methods. Estimates of the expected experimental values for the typically employed AGNR and laser parameters show that both the Rabi oscillations and multiphoton absorption are accessible in the laboratory. The data relevant to the intersubband tunneling makes the AGNR a 1D condensed matter analog in which the quantum electrodynamic vacuum decay can be detected by applying an external laboratory electric field.