The elusive quantum anomalous Hall effect in MnBi2Te4: a materials perspective

TL;DR

This paper reviews the challenges and potential strategies for realizing the quantum anomalous Hall effect in MnBi2Te4, emphasizing the importance of crystal quality, lattice imperfections, strain, and substrate interactions.

Contribution

It provides a materials perspective on tuning magnetic and topological properties of MnBi2Te4 to achieve QAHE, highlighting key factors influencing its realization.

Findings

Crystal quality is crucial for QAHE observation.

Lattice imperfections and strain can modify properties.

Substrate interactions impact magnetic and topological states.

Abstract

Observation of the quantum anomalous Hall effect (QAHE) in MnBi$_2$Te$_4$ flakes is one of the most exciting results in the study of the intrinsic magnetic topological insulator MnBi$_2$Te$_4$ and related compounds. This fascinating result is yet to be reproduced two years after its first report. The quality of starting MnBi$_2$Te$_4$ single crystals is believed to be the key factor. An interesting and important question to address is what is the right quality to enable the QAHE. In this perspective, we present possible approaches to tuning the magnetic and topological properties of MnBi$_2$Te$_4$ by using lattice imperfections, strain, stacking sequence, and interactions between the substrate and flakes/films. It is of critical importance to eventually identify the factor(s) responsible for the realization of QAHE.