Thermal Model for Time-Domain Thermoreflectance Experiments in a Laser Flash Geometry

TL;DR

This paper introduces a new thermal model for time-domain thermoreflectance experiments that can analyze front/back geometries where pump and probe beams irradiate opposite sides of a multilayer, expanding the interpretative capabilities beyond standard configurations.

Contribution

It presents a frequency-domain solution to the heat-diffusion equation for multilayers in front/back TDTR experiments, enabling analysis of new experimental geometries.

Findings

Model accurately predicts signals in front/back configurations.

Comparison shows differences between front/front and front/back geometries.

Experimental data agrees with model predictions.

Abstract

Time-domain thermoreflectance (TDTR) is a well-established pump/probe method for measuring thermal conductivity and interface conductance of multilayers. Interpreting signals in a TDTR experiment requires a thermal model.In standard front/front TDTR experiments, both pump and probe beams typically irradiate the surface of a multilayer. As a result, existing thermal models for interpreting thermoreflectance experiments assume the pump and probe beams both interact with the surface layer. Here, we present a frequency-domain solution to the heat-diffusion equation of a multilayer in response to nonhomogenous laser heating. This model allows analysis of experiments where the pump and probe beams irradiate opposite sides of a multilayer. We call such a geometry a front/back experiment to differentiate such experiments from standard TDTR experiments. As an example, we consider a 60nm amorphous Si film. We consider how signals differ in a front/front vs. front/back geometry and compare thermal model predictions to experimental data.