Microstructure, Surface Plasmon, Magneto-optic Surface Plasmon, and Sensitivity Properties of Magneto-plasmonic Co/Au Multilayers

TL;DR

This study investigates the microstructure and plasmonic properties of Co/Au multilayers, demonstrating enhanced sensor sensitivity through optimized multilayer design and excitation wavelength, with potential for improved detection limits.

Contribution

It provides detailed microstructural analysis of Co/Au multilayers and shows how tuning parameters enhances magneto-plasmonic sensor sensitivity.

Findings

Surface plasmon resonance sensitivity increased over 4 times at 785 nm wavelength.

Microstructure dominated by fcc-Au (111) layers.

Annealing affects strain and surface roughness.

Abstract

Microstructure properties of Co/Au multilayers prepared using dc-magnetron sputtering is reported using X-ray reflectivity (XRR) and X-ray diffraction (XRD) analysis. XRR profiles of these multilayers showed excellent bilayer periodicity. The XRD spectra displayed Co layer thickness-dependent properties. However, annealing increased lateral tensile strain decreased compressive strain along the normal substrate direction. While surface roughness, crystallite grain size, and strain are affected by Co layer thickness, microstructure and periodicity are dominated by fcc-Au (111). Surface plasmon resonance (SPR) and magneto-optic SPR study of an optimized Co/Au multilayer in Kretschmann configuration for air-He and water-Methanol media showed an enhanced sensitivity by over 4 times when excited at the wavelength of 785 nm as compared to the conventional SPR configuration when excited at the wavelength of 632.8 nm. This enhancement in MOSPR sensitivity means the detection limit of this class of transducers can be substantially improved by tuning Co/Au layer thickness, wavelength, and incident angle of optical radiation.