Introduction to theory of high-harmonic generation in solids: tutorial

TL;DR

This tutorial introduces the theoretical framework of high-harmonic generation in solids, covering microscopic dynamics, semiclassical models, and gauge choices, essential for understanding and modeling ultrafast laser-solid interactions.

Contribution

It provides a comprehensive, hands-on overview of theoretical approaches to HHG in solids, including gauge considerations and the role of the Berry phase, enhancing understanding of strong-field interactions.

Findings

Detailed description of microscopic dynamics approaches

Discussion of gauge choices and their implications

Overview of semiclassical recollision model

Abstract

High-harmonic generation (HHG) in solids has emerged in recent years as a rapidly expanding and interdisciplinary field, attracting attention from both the condensed-matter and the atomic, molecular, and optics communities. It has exciting prospects for the engineering of new light sources and the probing of ultrafast carrier dynamics in solids, and the theoretical understanding of this process is of fundamental importance. This tutorial provides a hands-on introduction to the theoretical description of the strong-field laser-matter interactions in a condensed-phase system that give rise to HHG. We provide an overview ranging from a detailed description of different approaches to calculating the microscopic dynamics and how these are intricately connected to the description of the crystal structure, through the conceptual understanding of HHG in solids as supported by the semiclassical recollision model, and finally a brief description of how to calculate the macroscopic response. We also give a general introduction to the Berry phase, and we discuss important subtleties in the modelling of HHG, such as the choice of structure and laser gauges, and the construction of a smooth and periodic structure gauge for both nondegenerate and degenerate bands. The advantages and drawback of different structure and laser-gauge choices are discussed, both in terms of their ability to address specific questions and in terms of their numerical feasibility.