Observations of Ultrafast Superfluorescent Beatings in a Cesium Atomic Vapor Excited by Femtosecond Laser Pulses

TL;DR

This study observes ultrafast superfluorescent beatings in cesium vapor excited by femtosecond laser pulses, revealing new insights into atomic coherence and emission dynamics on picosecond and femtosecond timescales.

Contribution

It reports the first observation of picosecond and femtosecond superfluorescent beatings involving both directly and indirectly excited atomic states in cesium vapor.

Findings

Superfluorescent blue light exhibits delayed buildup dependent on laser power and temperature.

Beatings with periods of 100 ps and 230 fs are observed, corresponding to atomic level splittings.

Control of superfluorescent beatings could enable rapid quantum operations.

Abstract

Spontaneous emission from individual atoms in vapor lasts nanoseconds, if not microseconds, and beatings in this emission involve only directly excited energy sublevels. In contrast, the superfluorescent emissions burst on a much-reduced timescale and their beatings involve both directly and indirectly excited energy sublevels. In this work, picosecond and femtosecond superfluorescent beatings are observed from a dense cesium atomic vapor. Cesium atoms are excited by 60-femtosecond long, 800 nm laser pulses via two-photon processes into their coherent superpositions of the ground 6S and excited 8S states. As a part of the transient four wave mixing process, the yoked superfluorescent blue light at lower transitions of 6S - 7P are recorded and studied. Delayed buildup time of this blue light is measured as a function of the input laser beam power using a high-resolution 2 ps streak camera. The power dependent buildup delay time is consistently doubled as the vapor temperature is lowered to cut the number of atoms by half. At low power and density, a beating with a period of 100 picoseconds representing the ground state splitting is observed. The autocorrelation measurements of the generated blue light exhibit a beating with a quasi-period of 230 fs corresponding to the splitting of the 7P level primarily at lower input laser power. Understanding and, eventually, controlling the intriguing nature of superfluorescent beatings may permit a rapid quantum operation free from the rather slow spontaneous emission processes from atoms and molecules.