Brillouin Light Scattering from Quantized Spin Waves in Nanowires with Antisymmetric Exchange Interactions

TL;DR

This study investigates how antisymmetric exchange interactions, specifically Dzyaloshinskii-Moriya interactions, influence spin wave behavior in nanowires, revealing non-reciprocal propagation and quantization effects through Brillouin light scattering experiments.

Contribution

It provides experimental evidence and a theoretical model showing the impact of Dzyaloshinskii-Moriya interactions on confined spin waves in nanostructures.

Findings

Frequency shift reduction in narrow wires for transverse scattering

Frequency shift independence for longitudinal propagating spin waves

Model accurately predicts the observed physics

Abstract

Antisymmetric exchange interactions lead to non-reciprocal spin-wave propagation. As a result, spin waves confined in a nanostructure are not standing waves; they have a time-dependent phase, because counter-propagating waves of the same frequency have different wavelengths. We report on a Brillouin light scattering (BLS) study of confined spin waves in Co/Pt nanowires with strong Dzyaloshinskii-Moriya interactions (DMI). Spin-wave quantization in narrow ($\lesssim 200$ nm width) wires dramatically reduces the frequency shift between BLS Stokes and anti-Stokes lines associated with the scattering of light incident transverse to the nanowires. In contrast, the BLS frequency shift associated with the scattering of spin waves propagating along the nanowire length is independent of nanowire width. A model that considers the chiral nature of modes captures this physics and predicts a dramatic reduction in frequency shift of light scattered from higher energy spin waves in narrow wires, which is confirmed by our experiments.