Non-Abelian statistics in light scattering processes across interacting Haldane chains

TL;DR

This paper explores non-Abelian statistics in light scattering of Haldane chains, revealing unconventional scattering phenomena linked to topological states and fractionalization effects induced by light.

Contribution

It proposes that light-induced interchain exchange processes cause fractionalization in topologically trivial Haldane chains, suggesting a mechanism for non-Abelian statistics in such systems.

Findings

Observation of mixed bosonic/fermionic statistics in scattering

Identification of light-induced interchain exchange processes

Comparison with SrCo₂V₂O₈ supports the proposed mechanism

Abstract

The $S=1$ Haldane state is constructed from a product of local singlet dimers in the bulk and topological states at the edges of a chain. It is a fundamental representative of topological quantum matter. Its well-known representative, the quasi-one-dimensional SrNi$_2$V$_2$O$_8$ shows both conventional as well as unconventional magnetic Raman scattering. The former is observed as one- and two-triplet excitations with small linewidths and energies corresponding to the Haldane gap $\Delta_H$ and the exchange coupling $J_c$ along the chain, respectively. Well-defined magnetic quasiparticles are assumed to be stabilized by interchain interactions and uniaxial single-ion anisotropy. Unconventional scattering exists as broad continua of scattering with an intensity $I(T)$ that shows a mixed bosonic / fermionic statistic. Such a mixed statistic has also been observed in Kitaev spin liquids and could point to a non-Abelian symmetry. As the ground state in the bulk of SrNi$_2$V$_2$O$_8$ is topologically trivial, we suggest its fractionalization to be due to light-induced interchain exchange processes. These processes are supposed to be enhanced due to a proximity to an Ising ordered state with a quantum critical point. A comparison with SrCo$_2$V$_2$O$_8$, the $S=1/2$ analogue to our title compound, supports these statements.