Unusual competition of superconductivity and charge-density-wave state in a compressed topological kagome metal

TL;DR

This study reveals an unusual double-peak pressure dependence of superconductivity in CsV3Sb5, highlighting a complex competition between superconductivity and charge-density-wave states influenced by pressure.

Contribution

It uncovers a novel double-peak behavior of Tc under pressure and demonstrates the complex interplay between superconductivity and CDW in a topological kagome metal.

Findings

Superconductivity shows a double-peak behavior with pressure.

Charge-density-wave state is suppressed at around 2 GPa.

Unusual competition between superconductivity and CDW is observed.

Abstract

Understanding the competition between superconductivity and other ordered states (such as antiferromagnetic or charge-density-wave (CDW) state) is a central issue in condensed matter physics. The recently discovered layered kagome metal AV3Sb5 (A = K, Rb, and Cs) provides us a new playground to study the interplay of superconductivity and CDW state by involving nontrivial topology of band structures. Here, we conduct high-pressure electrical transport and magnetic susceptibility measurements to study CsV3Sb5 with the highest Tc of 2.7 K in AV3Sb5 family. While the CDW transition is monotonically suppressed by pressure, superconductivity is enhanced with increasing pressure up to P1~0.7 GPa, then an unexpected suppression on superconductivity happens until pressure around 1.1 GPa, after that, Tc is enhanced with increasing pressure again. The CDW is completely suppressed at a critical pressure P2~2 GPa together with a maximum Tc of about 8 K. In contrast to a common dome-like behavior, the pressure-dependent Tc shows an unexpected double-peak behavior. The unusual suppression of Tc at P1 is concomitant with the rapidly damping of quantum oscillations, sudden enhancement of the residual resistivity and rapid decrease of magnetoresistance. Our discoveries indicate an unusual competition between superconductivity and CDW state in pressurized kagome lattice.