Strain-induced time reversal breaking and half quantum vortices near a putative superconducting tetra-critical point in Sr$_2$RuO$_4$

TL;DR

This paper investigates how spatially varying strain near a tetra-critical point in Sr$_2$RuO$_4$ can induce complex superconducting states, including time-reversal symmetry breaking and half-quantum vortices, reconciling theory with experiments.

Contribution

It provides a combined Landau-Ginzburg and microscopic analysis showing strain-induced textures and TRS-breaking states in Sr$_2$RuO$_4$, explaining experimental anomalies.

Findings

Strain induces $d \, ext{±} \, g$ states preserving TRS.

Domain walls can break TRS, forming $d+ig$ states.

Spatial strain patterns generate half-quantum fluxoids.

Abstract

It has been shown [1] that many seemingly contradictory experimental findings concerning the superconducting state in Sr$_2$RuO$_4$ can be accounted for as resulting from the existence of an assumed tetra-critical point at near ambient pressure at which $d_{x^2-y^2}$ and $g_{xy(x^2-y^2)}$ superconducting states are degenerate. We perform both a Landau-Ginzburg and a microscopic mean-field analysis of the effect of spatially varying strain on such a state. In the presence of finite $xy$ shear strain, the superconducting state consists of two possible symmetry-related time-reversal symmetry (TRS) preserving states: $d \pm g$. However, at domain walls between two such regions, TRS can be broken, resulting in a $d+ig$ state. More generally, we find that various natural patterns of spatially varying strain induce a rich variety of superconducting textures, including half-quantum fluxoids. These results may resolve some of the apparent inconsistencies between the theoretical proposal and various experimental observations, including the suggestive evidence of half-quantum vortices [2]. [1] Steven A Kivelson, Andrew C Yuan, BJ Ramshaw, and Ronny Thomale, "A proposal for reconciling diverse experiments on the superconducting state in Sr$_2$RuO$_4$," npj Quantum Mater 5 (2020). [2] J Jang, DG Ferguson, V Vakaryuk, Raffi Budakian, SB Chung, PM Goldbart, and Y Maeno, "Observation of half-height magnetization steps in Sr$_2$RuO$_4$," Science 331, 186-188 (2011).