Theory of record thermopower near a finite temperature magnetic phase transition: IrMn

TL;DR

This paper develops a theoretical model explaining the pronounced peak in thermopower near a magnetic phase transition in IrMn, highlighting the role of spin fluctuations and their impact on thermoelectric properties.

Contribution

The study introduces a theory linking spin fluctuation scattering to thermopower peaks near magnetic transitions, matching experimental observations in IrMn heterostructures.

Findings

Thermopower exhibits a prominent peak near the transition temperature.

Electrical resistivity shows a narrow, low peak at the transition.

The peak magnitude aligns with experimental data for three-dimensional spin fluctuations.

Abstract

The effect of scattering of conduction electrons by dynamical spin fluctuations on the thermopower in metals near a thermal phase transition into an antiferromagnetic phase is considered. We are interested in a transition at room temperature, as has been studied in a heterostructure involving layers of IrMn. We show that the electrical resistivity exhibits a narrow but low peak at the transition, which may be difficult to detect on top of the main contributions induced by phonons and impurities. By contrast, the thermopower is found to exhibit a prominent peak both as a function of temperature T for fixed layer thickness tAFM and as a function of tAFM for fixed T: We conjecture that the transition temperature Tc is a function of both tAFM and the Fermi energy EF . Both dependencies give rise to a sharp peak of the thermopower as a function of T or tAFM near the transition. The estimated magnitude of the peak for the case of three-dimensional longitudinal spin fluctuations is in good agreement with experiment.