Phase coherence of pairs of Cooper pairs as quasi-long-range order of half-vortex pairs in a two-dimensional bilayer system

TL;DR

This paper investigates how second-order Josephson coupling in a 2D bilayer system can induce exotic superconducting phases, including charge-4e superconductivity, by analyzing phase coherence and topological order using tensor-network methods.

Contribution

It introduces a novel phase transition scenario in bilayer systems with second-order Josephson coupling, revealing the emergence of charge-4e superconductivity and quasi-long-range order of Cooper pair pairs.

Findings

Inter-layer Ising long-range order is established below the BKT transition.

An intermediate quasi-LRO phase appears in inequivalent layers, with half-vortex pairs.

Charge-4e superconductivity can be realized in the bilayer system.

Abstract

It is known that the loss of phase coherence of Cooper pairs in two-dimensional (2D) superconductivity corresponds to the unbinding of vortex-antivortex pairs with the quasi-long-range order (quasi-LRO) in the order-parameter phase field, described by the Berezinskii-Kosterlizt-Thouless (BKT) transition of a 2D XY model. Here we show that the second-order Josephson coupling can induce an exotic superconducting phase in a bilayer system. By using tensor-network methods, the partition function of the 2D classical model is expressed as a product of 1D quantum transfer operator, whose eigen-equation can be solved by an algorithm of matrix product states rigorously. From the singularity shown by the entanglement entropy of the 1D quantum analogue, various phase transitions can be accurately determined. Below the BKT phase transition, an inter-layer Ising long-range order is established at $T_{Ising}$, and the phase coherence of both intra-layers and inter-layers is locked together. For two identical layers, the Ising transition coincides with the BKT transition at a multi-critical point. For two inequivalent layers, however, there emerges an intermediate quasi-LRO phase ($T_{Ising}<T<T_{BKT}$), where the vortex-antivortex bindings occur in the layer with the larger intra-layer coupling, but only half-vortex pairs with topological strings exist in the other layer, corresponding to the phase coherence of pairs of Cooper pairs. So our study provides a promising way to realize the charge-4e superconductivity in a bilayer system.