A unified theory of spin and charge excitations in high-$T_c$ cuprates: Quantitative comparison with experiment and interpretation

TL;DR

This paper presents a unified theoretical framework for understanding spin and charge excitations in high-temperature cuprate superconductors, quantitatively matching experimental RIXS data across doping levels.

Contribution

It introduces a combined VWF+$1/ N_f$ approach within an extended Hubbard model to accurately describe collective excitations in cuprates.

Findings

Paramagnons persist from underdoped to overdoped regimes.

Plasmons show three-dimensional character with specific oscillation modes.

Theoretical energies semi-quantitatively match RIXS data.

Abstract

We provide a unified interpretation of both paramagnon and plasmon modes in high-$T_c$ copper-oxides, and verify it quantitatively against available resonant inelastic $x$-ray scattering (RIXS) data across the hole-doped phase diagram. Three-dimensional extended Hubbard model, with included long-range Coulomb interactions and doping-independent microscopic parameters for both classes of quantum fluctuations, is used. Collective modes are studied using VWF+$1/\mathcal{N}_f$ approach which extends variational wave function (VWF) scheme by means of an expansion in inverse number of fermionic flavors ($1/\mathcal{N}_f$). We show that intense paramagnons persist along the anti-nodal line from the underdoped to overdoped regime and undergo rapid overdamping in the nodal direction. Plasmons exhibit a three-dimensional character, with minimal energy corresponding to anti-phase oscillations on neighboring $\mathrm{CuO_2}$ planes. The theoretical spin- and charge excitation energies reproduce semi-quantitatively RIXS data for $\mathrm{(Bi, Pb)_2 (Sr, La)_2 CuO_{6+\delta}}$. The present VWF+$1/\mathcal{N}_f$ analysis of dynamics and former VWF results for static quantities combine into a consistent description of the principal properties of hole-doped high-$T_c$ cuprates as strongly correlated systems.