Strain engineering of topological magnons in chromium trihalides from first-principles

TL;DR

This paper uses first-principles calculations to demonstrate topological magnons in chromium trihalides monolayers, showing how strain can enhance the Dzyaloshinskii-Moriya interaction to control magnon gaps, advancing topological magnonics.

Contribution

It provides the first ab initio evidence of topological magnons in monolayer chromium trihalides and shows how strain engineering can tune their properties.

Findings

Confirmed the existence of a magnon gap at the K point in CrI3 due to DM interaction.

Demonstrated strain can enhance the DM interaction and increase the magnon gap.

Supported potential for designing topological magnonic devices using strain control.

Abstract

Recent experiments evidence the direct observation of spin waves in chromium trihalides and a gap at the Dirac points of the magnon dispersion in bulk CrI$_3$. However, the topological origin of this feature remains unclear and its emergence at the 2D limit has not yet been proven experimentally. Herein, we perform a fully self-consistent ab initio analysis that supports the presence of topological magnons in chromium trihalides monolayers. Our results confirm the existence of a gap around the K high-symmetry point in the linear magnon dispersion of CrI$_3$, which originates as a direct consequence of intralayer Dzyaloshinskii-Moriya (DM) interaction. In addition, our orbital resolved analysis reveals the microscopic mechanisms that can be exploited using strain engineering to increase the strength of the DM interaction and thus control the gap size in CrI$_3$. This paves the way to the further development of this family of materials as building-blocks for topological magnonics at the limit of miniaturization.