Light-matter coupling and quantum geometry in moir\'e materials

TL;DR

This paper explores the fundamental relations between light-matter coupling and quantum geometry in flat-band and moiré materials, revealing how geometric contributions enable strong coupling and topological effects despite vanishing band velocities.

Contribution

It establishes the connection between quantum geometry and light-matter interactions in flat-band systems, providing new insights and design principles for controlling electronic properties in moiré materials.

Findings

Quantum metric enables diamagnetic coupling in flat bands.

Berry connection governs inter-band dipole matrix elements.

Floquet-topological gaps can open at magic angles under circularly polarized light.

Abstract

Quantum geometry has been identified as an important ingredient for the physics of quantum materials and especially of flat-band systems, such as moir\'e materials. On the other hand, the coupling between light and matter is of key importance across disciplines and especially for Floquet and cavity engineering of solids. Here we present fundamental relations between light-matter coupling and quantum geometry of Bloch wave functions, with a particular focus on flat-band and moir\'e materials, in which the quenching of the electronic kinetic energy could allow one to reach the limit of strong light-matter coupling more easily than in highly dispersive systems. We show that, despite the fact that flat bands have vanishing band velocities and curvatures, light couples to them via geometric contributions. Specifically, the intra-band quantum metric allows diamagnetic coupling inside a flat band; the inter-band Berry connection governs dipole matrix elements between flat and dispersive bands. We illustrate these effects in two representative model systems: (i) a sawtooth quantum chain with a single flat band, and (ii) a tight-binding model for twisted bilayer graphene. For (i) we highlight the importance of quantum geometry by demonstrating a nonvanishing diamagnetic light-matter coupling inside the flat band. For (ii) we explore the twist-angle dependence of various light-matter coupling matrix elements. Furthermore, at the magic angle corresponding to almost flat bands, we show a Floquet-topological gap opening under irradiation with circularly polarized light despite the nearly vanishing Fermi velocity. We discuss how these findings provide fundamental design principles and tools for light-matter-coupling-based control of emergent electronic properties in flat-band and moir\'e materials.