Understanding the role of exchange and correlations in complex oxides under strain and oxide heterostructures

TL;DR

This paper reviews how exchange and correlation effects influence the emergence of exotic electronic phases in complex oxides under strain and in heterostructures, highlighting recent theoretical advances and their implications for oxide electronics.

Contribution

It provides a comprehensive overview of theoretical studies on the role of exchange and correlations in complex oxides under strain and heterostructures, emphasizing their impact on exotic phases.

Findings

Correlation effects are crucial for understanding emergent phenomena in oxides.

Strain and heterostructures can induce novel electronic states.

Advanced first-principles methods help predict exotic phases.

Abstract

The study of complex oxides and oxide heterostructures have dominated the field of experimental and theoretical condensed matter research for the better part of the last few decades. Powerful experimental techniques like molecular beam epitaxy and pulsed laser deposition have made fabrication of oxide heterostructures with atomically sharp interfaces possible, while more and more sophisticated handling of exchange and correlations within first principles methods including density functional theory (DFT) supplemented with Hubbard U corrections and hybrid functionals, and beyond DFT techniques like dynamical mean field theory (DMFT) have made understanding of such correlated oxides and oxide interfaces easier. The emergence of the high mobility two dimensional electron gas with fascinating properties like giant photoconductance, large negative magnetoresistance, superconductivity, ferromagnetism, and the mysterious coexistence of the latter two have indeed caught the attention of condensed matter community at large. Similarly strain tuning of oxides have generated considerable interest particularly after the recent discovery of piezoelectric methods of strain generation. Theoretical understanding and prediction of the possible exotic phases emerging in such complex oxides both under strain and in heterostructures will eventually lead to better design of device applications in this new emerging field of oxide electronics, along with possible discovery of exotic physics in condensed matter systems which may be of wider significance! In this review we briefly look at theoretical studies of novel phenomena in oxides under strain and oxide heterostructures, and try to understand the role of exchange and particularly correlation in giving rise to such exotic electronic states.