Dissecting Sub-Cycle Interference in Photoelectron Holography

TL;DR

This paper advances photoelectron holography by combining novel data analysis techniques to suppress background effects, enabling detailed experimental-theoretical comparison and revealing sub-cycle electron dynamics with high precision.

Contribution

It introduces unit-cell averaging and time-filtering methods that improve the resolution of sub-cycle interference patterns in strong-field ionization experiments.

Findings

Suppression of ATI rings enhances holographic fringe clarity

High-precision match between experiment and CQSFA theory

Identification of interference pathways and phase differences

Abstract

Multipath holographic interference in strong-field quantum tunnel ionization is key to revealing sub-Angstrom attosecond dynamics for molecular movies. This critical sub-cycle motion is often obscured by longer time-scale effects such as ring-shaped patterns that appear in above-threshold ionization (ATI). In the present work, we overcome this problem by combining two novel techniques in theory and experimental analysis: unit-cell averaging and time-filtering data and simulations. Together these suppress ATI rings and enable an unprecedented highly-detailed quantitative match between strong-field ionization experiments in argon and the Coulomb-quantum orbit strong-field approximation (CQSFA) theory. Velocity map images reveal fine modulations on the holographic spider-like interference fringes that form near the polarization axis. CQSFA theory traces this to the interference of three types of electron pathways. The level of agreement between experiment and theory allows sensitive determination of quantum phase differences and symmetries, providing an important tool for quantitative dynamical imaging in quantum systems.