Superconducting state of Sr$_2$RuO$_4$ in the presence of longer-range Coulomb interactions

TL;DR

This study investigates the superconducting pairing symmetry of Sr$_2$RuO$_4$, considering longer-range Coulomb interactions, and finds that mixed $s'+id_{xy}$ or $s'+ip$ states best match experimental observations.

Contribution

It provides a detailed microscopic analysis showing that longer-range Coulomb interactions favor nodal mixed states over previously proposed pairing symmetries in Sr$_2$RuO$_4$.

Findings

Nodal $s'+id_{xy}$ state aligns with experimental data.

Longer-range Coulomb interactions favor mixed pairing states.

$g$- and $d_{x^2-y^2}$-wave channels are less competitive.

Abstract

The symmetry of the superconducting condensate in Sr$_2$RuO$_4$ remains controversial after nuclear magnetic resonance (NMR) experiments recently overturned the dominant chiral $p$-wave paradigm. Several theoretical proposals have been put forward to account for existing experiments, including a $d+ig$-wave admixture, conjectured to be stabilized by longer-range Coulomb interactions. We perform a material-specific microscopic theoretical study of pairing by spin- and charge-fluctuations in Sr$_2$RuO$_4$, including the effects of spin-orbit coupling, and both local and longer-range Coulomb repulsion. The latter has important consequences for Sr$_2$RuO$_4$ due to the near-degeneracy of symmetry-distinct pairing states in this material. We find that both the $g$- and $d_{x^2-y^2}$-wave channels remain noncompetitive compared to leading nodal $s'$, $d_{xy}$, and helical ($p$) solutions. This suggests nodal time-reversal symmetry broken $s'+id_{xy}$ or $s'+ip$ phases, promoted by longer-range Coulomb repulsion, as the most favorable candidates for Sr$_2$RuO$_4$. We analyse the properties of these states, and show that the $s'+id_{xy}$ solution agrees with the bulk of available experimental data, including recent discoveries from NMR, muon spin relaxation ($\mu$SR), and ultrasound measurements.