New $\alpha$-Emitting Isotope $^{214}$U and Abnormal Enhancement of $\alpha$-Particle Clustering in Lightest Uranium Isotopes

TL;DR

This paper reports the discovery of a new alpha-emitting isotope $^{214}$U, measures its decay properties, and finds an unexpected enhancement in alpha clustering linked to proton-neutron interactions, supported by shell model calculations.

Contribution

The study introduces the first identification of $^{214}$U and reveals an abnormal alpha clustering enhancement in light uranium isotopes due to monopole proton-neutron interactions.

Findings

Discovery of $^{214}$U isotope via fusion-evaporation reaction.

Significant enhancement of alpha decay reduced widths in $^{214}$U and $^{216}$U.

Shell model calculations support the role of monopole interactions in alpha clustering.

Abstract

A new $\alpha$-emitting isotope $^{214}$U, produced by fusion-evaporation reaction $^{182}$W($^{36}$Ar, 4n)$^{214}$U, was identified by employing the gas-filled recoil separator SHANS and recoil-$\alpha$ correlation technique. More precise $\alpha$-decay properties of even-even nuclei $^{216,218}$U were also measured in reactions of $^{40}$Ar, $^{40}$Ca with $^{180, 182, 184}$W targets. By combining the experimental data, improved $\alpha$-decay reduced widths $\delta^2$ for the even-even Po--Pu nuclei in the vicinity of magic neutron number $N=126$ were deduced. Their systematic trends are discussed in terms of $N_{p}N_{n}$ scheme in order to study the influence of proton-neutron interaction on $\alpha$ decay in this region of nuclei. It is strikingly found that the reduced widths of $^{214,216}$U are significantly enhanced by a factor of two as compared with the $N_{p}N_{n}$ systematics for the $84 \leq Z \leq 90$ and $N<126$ even-even nuclei. The abnormal enhancement is interpreted by the strong monopole interaction between the valence protons and neutrons occupying the $\pi 1f_{7/2}$ and $\nu 1f_{5/2}$ spin-orbit partner orbits, which is supported by a large-scale shell model calculation.