On the shear-driven surfactant layer instability

TL;DR

This study experimentally investigates the flow patterns caused by shear-driven surfactant layers at water surfaces, introducing a new non-dimensional parameter called the surface Rayleigh number to describe flow instabilities.

Contribution

The paper develops a unified approach to describe flow patterns using two non-dimensional parameters, including the newly introduced surface Rayleigh number, for shear-driven surfactant layer instability.

Findings

Flow patterns are governed by two key non-dimensional parameters.

The surface Rayleigh number predicts multi-vortex flow structures.

Critical conditions for surfactant layer instability are identified.

Abstract

The structure and stability of the convective flow generated by a source located at the water surface containing an insoluble surfactant layer are experimentally investigated. Application of a few types of source, which differ in the force driving the interface, and two surfactants with different rheological properties made it possible to generalize the results and to develop a unified approach to describing the flow patterns observed in this study. It is shown that, regardless of source type and surfactant used, the problem under consideration can be completely described in terms of two non-dimensional parameters. The first is the elasticity number introduced earlier by Homsy and Meiburg (J. Fluid Mech., v.139, 1984). This parameter is the ratio of two shear stresses formed at the interface by surfactant and source, and it defines the formation of the convective zone at the center nearby the source and the size of the stagnant zone at the periphery. The second, called the surface Rayleigh number, is introduced for the first time in this paper. It is responsible for the appearance of the multi-vortex flow structure within the stagnant zone. We suppose that this structure occurs as a result of the mechanical equilibrium instability of the surfactant layer under the action of the momentum flux transported from the subphase by the viscous mechanism. Based on our results and those reported earlier by other researchers, we have determined the critical value of the surface Rayleigh number and analyzed the possibility and conditions for the occurrence of this instability, called by us the shear-driven surfactant layer (SDSL) instability, by addressing some problems of interfacial hydrodynamics.