Magnetoexcitons in transition-metal dichalcogenides monolayers, bilayers, and van der Waals heterostructures

TL;DR

This study investigates how magnetic fields and layer configurations influence the binding energies and diamagnetic coefficients of magnetoexcitons in TMDC monolayers, bilayers, and heterostructures, revealing tunable excitonic properties.

Contribution

It introduces calculations of binding energies and diamagnetic coefficients for indirect magnetoexcitons in TMDC heterostructures, highlighting the role of screening and layer number in exciton control.

Findings

Magnetic field affects binding energies and DMCs of magnetoexcitons.

Layer number, especially hBN layers, tunes excitonic properties.

Screening effects are significant in heterostructure exciton behavior.

Abstract

We study direct and indirect magnetoexcitons in Rydberg states in monolayers and heterostructures of transition-metal dichalcogenices (TMDCs) in an external magnetic field, applied perpendicular to the monolayer or heterostructures. We calculate binding energies of magnetoexcitons for the Rydberg states 1$s$, 2$s$, 3$s$, and 4$s$ by numerical integration of the Schr\"{o}dinger equation using the Rytova-Keldysh potential for direct magnetoexcitons and both the Rytova-Keldysh and Coulomb potentials for indirect magnetoexcitons. Latter allows understanding the role of screening in TMDCs heterostructures. We report the magnetic field energy contribution to the binding energies and diamagnetic coefficients (DMCs) for direct and indirect magnetoexcitons. The tunability of the energy contribution of direct and indirect magnetoexcitons by the magnetic field is demonstrated. It is shown that binding energies and DMCs of indirect magnetoexcitons can be manipulated by the number of hBN layers. Therefore, our study raises the possibility of controlling the binding energies of direct and indirect magnetostrictions in TMDC monolayers, bilayers and heterostructures using magnetic field and opens an additional degree of freedom to tailor the binding energies and DMCs for heterostructures by varying the number of hBN sheets between TMDC layers. The calculations of the binding energies and DMCs of indirect magnetoexcitons in TMDC heterostructures are novel and can be compared with the experimental results when they will be available.