Non-local magnon-based transport in yttrium iron garnet/platinum heterostructures at high temperatures

TL;DR

This study investigates the temperature-dependent spin Hall and magnon-mediated magnetoresistance in yttrium iron garnet/platinum heterostructures, revealing how high temperatures affect magnetic and electronic transport properties.

Contribution

It provides new insights into the temperature evolution of non-local magnon transport and interface effects in YIG/Pt heterostructures up to and beyond the Curie temperature.

Findings

Spin Hall magnetoresistance decreases with temperature, vanishing near 500 K.

Non-local magnon-mediated magnetoresistance follows a temperature-dependent power law.

High-temperature offset voltage indicates electronic leakage related to band gap energy.

Abstract

The spin Hall effect in a heavy metal thin film allows to probe the magnetic properties of an adjacent magnetic insulator via magnetotransport measurements. Here, we investigate the magnetoresistive response of yttrium iron garnet/platinum heterostructures from room temperature to beyond the Curie temperature $T_\mathrm{C, YIG} \approx 560\,\mathrm{K}$ of the ferrimagnetic insulator. We find that the amplitude of the (local) spin Hall magnetoresistance decreases monotonically from $300\,\mathrm{K}$ towards $T_\mathrm{C}$, mimicking the evolution of the saturation magnetization of yttrium iron garnet. Interestingly, the spin Hall magnetoresistance vanishes around $500\,\mathrm{K}$, well below $T_\mathrm{C}$, which we attribute to the formation of a parasitic interface layer by interdiffusion. Around room temperature the non-local magnon-mediated magnetoresistance exhibits a power law scaling $T^{\alpha}$ with $\alpha = 3/2$, as already reported. The exponent decreases gradually to $\alpha \sim 1/2$ at around $420\,\mathrm{K}$, before the non-local magnetoresistance vanishes rapidly at a similar temperature as the spin Hall magnetoresistance. We attribute the reduced $\alpha$ at high temperatures to the increasing thermal magnon population which leads to enhanced scattering of the non-equilibrium magnon population and a reduced magnon diffusion length. Finally, we find a magnetic field independent offset voltage in the non-local signal for $T > 470\,\mathrm{K}$ which we associate with electronic leakage currents through the normally insulating yttrium iron garnet film. Indeed, this non-local offset voltage is thermally activated with an energy close to the band gap.