Detection of NaRb Feshbach molecule by photodissociation

TL;DR

This paper presents a novel method for detecting NaRb Feshbach molecules using photodissociation combined with absorption imaging, enabling in situ observation of molecular collision dynamics.

Contribution

The authors develop a new detection technique for NaRb Feshbach molecules that allows in situ, high-resolution measurement of molecular populations and dynamics.

Findings

Successful detection of NaRb Feshbach molecules via photodissociation.

Optimized detection protocol for measuring molecular temperature.

Demonstrated potential for studying collision dynamics in molecular gases.

Abstract

We demonstrate detection of NaRb Feshbach molecules at high magnetic field by combining molecular photodissociation and absorption imaging of the photofragments. The photodissociation process is carried out via a spectroscopically selected hyperfine Zeeman level correlated with the Na ($3P_{3/2}$) + Rb ($5S_{1/2}$) asymptote which, following spontaneous emission and optical pumping, leads to ground-state atoms in a single level with near unity probability. Subsequent to the dissociation, the number of molecules is obtained by detecting the resultant $^{23}$Na and $^{87}$Rb atoms. We have also studied the heating effect caused by the photodissociation process and optimized the detection protocol for extracting the temperature of the molecular cloud. This method enables the $in~situ$ detection of fast time scale collision dynamics between NaRb Feshbach molecules and will be a valuable capability in studying few-body physics involving molecules.