Coil-stretch-like transition of elastic sheets in extensional flows

TL;DR

This study demonstrates a coil-stretch-like transition in elastic sheets under extensional flows, revealing bistability between compact and stretched states influenced by elasticity models and hydrodynamic interactions.

Contribution

It introduces the concept of a coil-stretch-like transition in elastic sheets, showing how nonlinear elasticity and hydrodynamics lead to bistability in sheet conformations.

Findings

Bistability exists between compact and stretched states.

Nonlinear elasticity arrests unbounded stretching.

Hydrodynamic interactions are essential for bistability.

Abstract

The conformation of a long linear polymer dissolved in fluid and exposed to an extensional flow is well-known to exhibit a "coil-stretch" transition, which for sufficiently long chains can lead to bistability. The present work reports computations indicating that an analogous "compact-stretched" transition arises in the dynamics of a thin elastic sheet. Sheets of nominally circular, square or rectangular shape are simulated in planar and biaxial flows using a finite element method for the sheet conformations and a regularized Stokeslet method for the fluid flow. If a neo-Hookean constitutive model is used for the sheet elasticity, the sheets will stretch without bound once a critical extension rate, as characterized nondimensionally by a capillary number, is exceeded. Nonlinear elasticity, represented with the Yeoh model, arrests the stretching, leading to a highly-stretched steady state once the critical capillary number is exceeded. For all shapes and in both planar and biaxial extension, a parameter regime exists in which both weakly stretched (compact) and strongly stretched states can be found, depending on initial conditions. I.e. this parameter regime displays bistability. As in the long-chain polymer case, the bistable behavior arises from the hydrodynamic interaction between distant elements of the sheet, and vanishes if these interactions are artificially screened by use of a Brinkman model for the fluid motion. While the sheets can transiently display wrinkled shapes, all final shapes in planar and biaxial extension are planar.