Coincidence inelastic neutron scattering for detection of two-spin magnetic correlations

TL;DR

This paper introduces coincidence inelastic neutron scattering (cINS), a novel technique that enables direct detection of two-spin magnetic correlations in quantum magnets, surpassing the limitations of traditional INS.

Contribution

The paper proposes and theoretically analyzes cINS, a new neutron scattering method capable of directly measuring two-spin correlations in magnetic materials.

Findings

cINS can detect two-spin magnetic correlations explicitly.

It utilizes two neutron sources and detectors with coincidence detection.

Potential to study spin valence bond states in quantum magnets.

Abstract

Inelastic neutron scattering (INS) is one powerful technique to study the low-energy single-spin dynamics of magnetic materials. A variety of quantum magnets show novel magnetic correlations such as quantum spin liquids. These novel magnetic correlations are beyond the direct detection of INS. In this paper we propose a coincidence technique, coincidence inelastic neutron scattering (cINS), which can detect the two-spin magnetic correlations of the magnetic materials. In cINS there are two neutron sources and two neutron detectors with an additional coincidence detector. Two neutrons from the two neutron sources are incident on the target magnetic material, and they are scattered by the electron spins of the magnetic material. The two scattered neutrons are detected by the two neutron detectors in coincidence with the coincidence probability described by a two-spin Bethe-Salpeter wave function. Since the two-spin Bethe-Salpeter wave function defines the momentum-resolved dynamical wave function with two spins excited, cINS can explicitly detect the two-spin magnetic correlations of the magnetic material. Thus, it can be introduced to study the various spin valence bond states of the quantum magnets.