Control of Mooij correlations at the nanoscale in the disordered metallic Ta - nanoisland FeNi multilayers

TL;DR

This study investigates how nanoscale multilayered structures of disordered Ta and magnetic FeNi nanoislands exhibit localization phenomena affecting electronic transport, revealing effects below the MIR limit linked to quantum localization.

Contribution

It provides new insights into localization phenomena in disordered metallic multilayers and demonstrates how magnetic nanoisland layers influence electron delocalization and conductivity.

Findings

Localization causes reduced Drude response and new electronic excitations.

Increasing FeNi thickness leads to electron delocalization.

Discontinuous FeNi nanoislands cause conductivity below MIR limit.

Abstract

Localisation phenomena in highly disordered metals close to the extreme conditions determined by the Mott-Ioffe-Regel (MIR) limit when the electron mean free path is approximately equal to the interatomic distance is a challenging problem. Here, to shed light on these localisation phenomena, we studied the dc transport and optical conductivity properties of nanoscaled multilayered films composed of disordered metallic Ta and magnetic FeNi nanoisland layers, where ferromagnetic FeNi nanoislands have giant magnetic moments of 10^3-10^5 Bohr magnetons (\mu_B). In these multilayered structures, FeNi nanoisland giant magnetic moments are interacting due to the indirect exchange forces acting via the Ta electron subsystem. We discovered that the localisation phenomena in the disordered Ta layer lead to a decrease in the Drude contribution of free charge carriers and the appearance of the low-energy electronic excitations in the 1-2 eV spectral range characteristic of electronic correlations, which may accompany the formation of electronic inhomogeneities. From the consistent results of the dc transport and optical studies we found that with an increase in the FeNi layer thickness across the percolation threshold evolution from the superferromagnetic to ferromagnetic behaviour within the FeNi layer leads to the delocalisation of Ta electrons from the associated localised electronic states. On the contrary, we discovered that when the FeNi layer is discontinuous and represented by randomly distributed superparamagnetic FeNi nanoislands, the Ta layer normalized dc conductivity falls down below the MIR limit by about 60%. The discovered effect leading to the dc conductivity fall below the MIR limit can be associated with non-ergodicity and purely quantum (many-body) localisation phenomena, which need to be challenged further.