Magnetic Two-Dimensional Chromium Trihalides: A Theoretical Perspective

TL;DR

This paper reviews the current theoretical understanding of magnetic two-dimensional chromium trihalides, discussing their magnetic properties, open questions, recent predictions, and potential applications in future devices.

Contribution

It provides a comprehensive perspective on the theoretical insights into 2D chromium trihalides, highlighting well-established facts and addressing open issues and recent advances.

Findings

Understanding of magnetic moments and anisotropy in 2D Cr-trihalides

Discussion of open questions on spin couplings and magnon gaps

Recent theoretical predictions on Moiré magnets and skyrmions

Abstract

The discovery of ferromagnetic order in monolayer 2D crystals has opened a new venue in the field of two dimensional (2D) materials. 2D magnets are not only interesting on their own, but their integration in van der Waals heterostructures allows for the observation of new and exotic effects in the ultrathin limit. The family of Chromium trihalides, CrI$_3$, CrBr$_3$ and CrCl$_3$, is, so far, the most studied among magnetic 2D crystals. In this mini-review, we provide a perspective of the state of the art of the theoretical understanding of magnetic 2D trihalides, most of which will also be relevant for other 2D magnets, such as vanadium trihalides. We discuss both the well-established facts, such as the origin of the magnetic moment and magnetic anisotropy and address as well open issues such as the nature of the anisotropic spin couplings and the magnitude of the magnon gap. Recent theoretical predictions on Moir\' e magnets and magnetic skyrmions are also discussed. Finally, we give some prospects about the future interest of these materials and possible device applications.