Connecting Relaxation Time to a Dynamical Length Scale in Athermal Active Glass Formers

TL;DR

This study links the relaxation time to a dynamical length scale in active glass formers, revealing a scaling law that connects structural heterogeneity to slow dynamics across various active systems.

Contribution

It introduces a structural correlation-based length scale in active glasses and establishes a simple exponential scaling law for relaxation time involving this length scale.

Findings

Dynamical length scale $\xi$ correlates with slow particle clusters.

Relaxation time $ au_eta$ scales as $ ext{exp} (\xi \mu / T_{eff})$.

Results hold over three decades of persistence times.

Abstract

Supercooled liquids display dynamics that are inherently heterogeneous in space. This essentially means that at temperatures below the melting point, particle dynamics in certain regions of the liquid can be orders of magnitude faster than other regions. Often dubbed as dynamical heterogeneity, this behavior has fascinated researchers involved in the study of glass transition, for over two decades. A fundamentally important question in all glass transition studies is whether one can connect the growing relaxation time to a concomitantly growing length scale. In this paper, we go beyond the realm of ordinary glass forming liquids and study the origin of a growing dynamical length scale $\xi$ in a self propelled "active" glass former. This length scale which is constructed using structural correlations agrees well with the average size of the clusters of slow moving particles that are formed as the liquid becomes spatially heterogeneous. We further report that the concomitantly growing $\alpha$- relaxation time exhibits a simple scaling law, $\tau_\alpha \sim \text{exp} (\xi \mu / T_{eff})$, with $\mu$ as an effective chemical potential, $T_{eff}$ as the effective temperature, and $\xi \mu$ as the growing free energy barrier for cluster rearrangements. The findings of our study are valid over three decades of persistence times, and hence could be very useful in understanding the slow dynamics of a generic active liquid such as an active colloidal suspension, or a self propelled granular medium, to mention a few.