Four-wave mixing dynamics of a strongly coupled quantum-dot--microcavity system driven by up to 20 photons

TL;DR

This study combines experimental and theoretical approaches to analyze four-wave mixing dynamics in a quantum-dot microcavity system with up to 20 photons, confirming the Jaynes-Cummings model's applicability in this regime.

Contribution

It demonstrates the validity of the JC model for a strongly coupled quantum dot-microcavity system with a high photon number, including phonon effects and quasi-periodic FWM dynamics.

Findings

Excellent agreement between experiment and simulation.

FWM signals involve up to ~20 photons.

Observation of collapse and revival phenomena.

Abstract

The Jaynes-Cummings (JC) model represents one of the simplest ways in which single qubits can interact with single photon modes, leading to profound quantum phenomena like superpositions of light and matter states. One system, that can be described with the JC model, is a single quantum dot embedded in a micropillar cavity. In this joint experimental and theoretical study we investigate such a system using four-wave mixing (FWM) micro-spectroscopy. Special emphasis is laid on the dependence of the FWM signals on the number of photons injected into the microcavity. By comparing simulation and experiment, which are in excellent agreement with each other, we infer that up to ~20 photons take part in the observed FWM dynamics. Thus we verify the validity of the JC model for the system under consideration in this non-trivial regime. We find that the inevitable coupling between the quantum dot exciton and longitudinal acoustic phonons of the host lattice influences the real time FWM dynamics and has to be taken into account for a sufficient description of the quantum dot-microcavity system. Performing additional simulations in an idealized dissipation-less regime, we observe that the FWM signal exhibits quasi-periodic dynamics, analog to the collapse and revival phenomenon of the JC model. In these simulations we also see that the FWM spectrum has a triplet structure, if a large number of photons is injected into the cavity.