Gate-tunable exciton-polaron Rydberg series with strong roton effect

TL;DR

This paper reports the experimental observation of gate-tunable exciton polarons in monolayer MoSe2, revealing a Rydberg series with a strong roton effect and providing insights into complex many-body physics.

Contribution

It introduces the first observation of excited-state exciton polarons with a Rydberg series and roton-like dispersion in monolayer TMDs, expanding understanding of many-body quasiparticles.

Findings

Observation of gate-tunable exciton polarons in monolayer MoSe2.

Detection of a Rydberg series with increasing many-body effects.

Evidence of roton-like dispersion in exciton-polaron states.

Abstract

The electronic exciton polaron is a hypothetical many-body quasiparticle formed by an exciton dressed with a polarized electron-hole cloud in the Fermi sea (FS). It is predicted to display rich many-body physics and unusual roton-like dispersion. Exciton polarons were recently evoked to explain the excitonic spectra of doped monolayer transition metal dichalcogenides (TMDs), but these studies are limited to the ground state. Excited-state exciton polarons can exhibit richer many-body physics due to their larger spatial extent, but detection is challenging due to their inherently weak signals. Here we observe gate-tunable exciton polarons for the 1s - 3s excitonic Rydberg series in ultraclean monolayer MoSe$_2$ devices by optical spectroscopy. When the FS expands, we observe increasingly severe suppression and steep energy shift from low to high Rydberg states. Their gate-dependent energy shifts go beyond the trion description but match our exciton-polaron theory. Notably, the exciton-polaron absorption and emission bands are separated with an energy gap, which increases from ground to excited state. Such peculiar characteristics are attributed to the roton-like exciton-polaron dispersion, where energy minima occur at finite momenta. The roton effect increases from ground to excited state. Such exciton-polaron Rydberg series with progressively significant many-body and roton effect shall provide a new platform to explore complex many-body phenomena.